The 4K pack generally isn't the culprit on its own, unless it's from a sketchy source or corrupted. Most likely there's a conflict between that mod and another one you have installed, or the pack requires some dependency you're missing. That said, the most efficient way to figure it out is to disable EVERYTHING in your mod manager, confirm the game starts without issues, and then activate the mods in small blocks (for example, first just the texture pack, then half of the rest, etc.). That way you narrow down the problem using a binary approach instead of wasting hours testing one by one.
Besides disabling, clear the cache like they mentioned. But here's something nobody said: check the game logs. In the Starfield folder there should be error files, and sometimes they tell you exactly which mod is failing or what file it can't find. If the texture pack needs a specific version of some script mod or it's compressed badly, you'll see it there. Also, if the pack is really large (several GB), confirm your GPU has enough VRAM available; sometimes crashes with no message are from memory issues, not actual conflicts.